| Cite this article as: |
Ping Zhu, Pingping Wang, Puzhen Shao, Xiu Lin, Ziyang Xiu, Qiang Zhang, Equo Kobayashi, and Gaohui Wu, Research progress in interface modification and thermal conduction behavior of diamond/metal composites, Int. J. Miner. Metall. Mater., 29(2022), No. 2, pp. 200-211. https://doi.org/10.1007/s12613-021-2339-6
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王平平 E-mail: hit_wangpingping@163.com
修子扬 E-mail: xiuzy@hit.edu.cn
张强 E-mail: zhang_tsiang@hit.edu.cn
金刚石/金属复合材料以其优异的导热性能和低膨胀性能被广泛应用于航空航天和电子封装领域。然而，化学性能的差异导致金刚石与金属的界面不相容，这对复合材料的性能有很大的影响。为了提高金刚石与金属的界面相容性，必须对复合材料的界面进行改性。本文系统的总结了近年来金刚石/金属复合材料及其界面结构优化和性能控制在热管理领域的重要研究进展。介绍了近年来计算模拟技术在金刚石/金属复合材料研究中的应用。金刚石/金属界面改性主要通过基体金属合金化、金刚石颗粒表面处理及界面构型设计三种方式实现。其中，界面相的组成及尺寸是影响复合材料热性能的关键因素。此外，通过复合材料界面构型设计，在材料内部形成连续的金刚石颗粒导热通道为提高复合材料热导率提供了新的思路。近年来，在优化金刚石/金属界面结构的同时，研究者们也通过计算模拟对复合材料的界面性质及导热行为展开了研究。虽然已有针对金刚石/金属界面改性的大量研究，复合材料导热机制的理论研究尚不完善，应进一步建立金刚石/金属复合材料界面相组成和比例与导热系数之间的定量关系，为实验提供理论指导。此外，今后还可以借助多尺度模拟技术和实验研究金刚石/金属复合材料的界面结合和热传导机理。
Diamond/metal composites are widely used in aerospace and electronic packaging fields due to their outstanding high thermal conductivity and low expansion. However, the difference in chemical properties leads to interface incompatibility between diamond and metal, which has a considerable impact on the performance of the composites. To improve the interface compatibility between diamond and metal, it is necessary to modify the interface of composites. This paper reviews the experimental research on interface modification and the application of computational simulation in diamond/metal composites. Combining computational simulation with experimental methods is a promising way to promote diamond/metal composite interface modification research.
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