全固态锂电池中高镍三元材料的电化学性能及界面问题综述

王晶; 赵尚骞; 唐玲; 韩富娟; 张一; 夏一冕; 王力军; 卢世刚

doi:10.1007/s12613-022-2453-0

Volume 29 Issue 5

Apr. 2022

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文章导航 > 矿物冶金与材料学报（英文） > 2022 > 29(5): 1003-1018

Jing Wang, Shangqian Zhao, Ling Tang, Fujuan Han, Yi Zhang, Yimian Xia, Lijun Wang, and Shigang Lu, Review of the electrochemical performance and interfacial issues of high-nickel layered cathodes in inorganic all-solid-state batteries, Int. J. Miner. Metall. Mater., 29(2022), No. 5, pp. 1003-1018. https://doi.org/10.1007/s12613-022-2453-0

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Jing Wang, Shangqian Zhao, Ling Tang, Fujuan Han, Yi Zhang, Yimian Xia, Lijun Wang, and Shigang Lu, Review of the electrochemical performance and interfacial issues of high-nickel layered cathodes in inorganic all-solid-state batteries, Int. J. Miner. Metall. Mater., 29(2022), No. 5, pp. 1003-1018. https://doi.org/10.1007/s12613-022-2453-0

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特约综述

全固态锂电池中高镍三元材料的电化学性能及界面问题综述

1)
有研科技集团有限公司国家动力电池创新中心，北京 100088，中国
2)
国联汽车动力电池研究院有限责任公司，北京 100088，中国
3)
北京有色金属研究总院，北京 100088，中国
4)
上海大学材料基因组工程研究院，上海 200444，中国

通讯作者:
卢世刚 E-mail: lusg8867@163.com

文章亮点

(1) 分析了高镍三元材料在全固态电池与传统液体电池的电化学性能差异。

(2) 讨论了不同制备工艺对全固态电池电化学性能的影响，并给出了制备复合电极的建议。

(3) 从高镍三元材料与无机固态电解质界面总结了影响全固态电池中电化学性能的原因。

(4) 提出高镍三元材料在全固态电池中的应用方向和前景。

中文摘要

全固态电池在高比能量和高安全性方面有很大潜力，这成为了下一代锂离子电池的发展方向之一。然而全固态电池中，高镍三元材料和无机固体电解质的匹配有待解决。本综述总结了全固态电池中高镍三元材料和无机固体电解质在充放电和循环过程中的界面反应以及机械接触问题。本文提出，高镍三元材料和无机固体电解质在空间上的均匀接触以及固体电解质的离子传导性是影响高镍三元材料性能的重要因素。并指出复合电极中的高镍三元材料和固体电解质之间的界面反应和接触损耗直接影响了离子和电子进入活性材料的通道。因此，在高镍三元材料表面构建缓冲层可以防止活性材料和电解质之间的直接接触，减缓它们的界面反应。适当的缓冲层也可以通过减少高镍三元材料在充放电过程中的体积变化来减缓界面接触损失。最后，为实现高镍三元材料全固态电池的发展愿景，我们提出了以下建议：（1）开发高镍三元材料和无机固体电解质的电化学体系；（2）阐明高镍三元材料和无机固体电解质之间的界面和电极过程的基础科学，阐明两种材料之间的界面化学和电化学反应的机制，并解决内在的安全问题；（3）加强对高镍三元材料和固体电解质复合电极的工程技术及其制备方法的开发，促进全固态电池的产业化。

关键词:

Invited Review

Review of the electrochemical performance and interfacial issues of high-nickel layered cathodes in inorganic all-solid-state batteries

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Abstract

Abstract

All-solid-state batteries potentially exhibit high specific energy and high safety, which is one of the development directions for next-generation lithium-ion batteries. The compatibility of all-solid composite electrodes with high-nickel layered cathodes and inorganic solid electrolytes is one of the important problems to be solved. In addition, the interface and mechanical problems of high-nickel layered cathodes and inorganic solid electrolyte composite electrodes have not been thoroughly addressed. In this paper, the possible interface and mechanical problems in the preparation of high-nickel layered cathodes and inorganic solid electrolytes and their interface reaction during charge–discharge and cycling are reviewed. The mechanical contact problems from phenomena to internal causes are also analyzed. Uniform contact between the high-nickel cathode and solid electrolyte in space and the ionic conductivity of the solid electrolyte are the prerequisites for the good performance of a high-nickel layered cathode. The interface reaction and contact loss between the high-nickel layered cathode and solid electrolyte in the composite electrode directly affect the passage of ions and electrons into the active material. The buffer layer constructed on the high-nickel cathode surface can prevent direct contact between the active material and electrolyte and slow down their interface reaction. An appropriate protective layer can also slow down the interface contact loss by reducing the volume change of the high-nickel layered cathode during charge and discharge. Finally, the following recommendations are put forward to realize the development vision of high-nickel layered cathodes: (1) develop electrochemical systems for high-nickel layered cathodes and inorganic solid electrolytes; (2) elucidate the basic science of interface and electrode processes between high-nickel layered cathodes and inorganic solid electrolytes, clarify the mechanisms of the interfacial chemical and electrochemical reactions between the two materials, and address the intrinsic safety issues; (3) strengthen the development of research and engineering technologies and their preparation methods for composite electrodes with high-nickel layered cathodes and solid electrolytes and promote the industrialization of all-solid-state batteries.
- all-solid-state lithium-ion battery;
- high-nickel layered cathode;
- inorganic solid-state electrolyte;
- cathodes and electrolyte interface

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