综述：基于热解MOF衍生物的电磁波吸收剂

王秋怡; 刘杰; 李亚东; 娄志超; 李延军

doi:10.1007/s12613-022-2562-9

Volume 30 Issue 3

Mar. 2023

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文章导航 > 矿物冶金与材料学报（英文） > 2023 > 30(3): 446-473

Qiuyi Wang, Jie Liu, Yadong Li, Zhichao Lou, and Yanjun Li, A literature review of MOF derivatives of electromagnetic wave absorbers mainly based on pyrolysis, Int. J. Miner. Metall. Mater., 30(2023), No. 3, pp. 446-473. https://doi.org/10.1007/s12613-022-2562-9

Cite this article as:

Qiuyi Wang, Jie Liu, Yadong Li, Zhichao Lou, and Yanjun Li, A literature review of MOF derivatives of electromagnetic wave absorbers mainly based on pyrolysis, Int. J. Miner. Metall. Mater., 30(2023), No. 3, pp. 446-473. https://doi.org/10.1007/s12613-022-2562-9

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特约综述

综述：基于热解MOF衍生物的电磁波吸收剂

1)
南京林业大学江苏省林业资源高效加工利用协同创新中心, 江苏南京 210037
2)
南京林业大学材料科学与工程学院, 江苏南京 210037
3)
河南省对外科技交流中心, 河南郑州 450000
4)
College of Engineering, University of Georgia, Athens 30605, USA

通讯作者:
娄志超 E-mail: zc-lou2015@njfu.edu.cn

李延军 E-mail: nfcm2018@163.com

文章亮点

(1) 系统地总结了基于热解MOF衍生物的电磁波吸收剂的研究现状。

(2) 详细地描述了制备MOF衍生EMW吸波材料的电磁(EM)能量耗散机理和策略。

(3) 提出了调整MOF衍生物的电磁参数的方法。

中文摘要

日益严重的电磁污染多年来一直困扰着电磁能量耗散领域的研究人员，有效地解决这一问题变得越来越重要。金属有机骨架(MOF)作为功能材料中的一颗璀璨之星，因其具有高度可调的孔隙率、结构和通用性等优点而备受关注。MOF衍生的电磁波(EMW)吸波材料具有重量轻、匹配厚度薄、容量大、有效带宽宽等优点，被广泛报道。然而，目前的研究缺乏基于热解MOF衍生物的电磁波吸收剂的系统总结。在这里，我们详细地描述了制备MOF衍生EMW吸波材料的电磁(EM)能量耗散机理和策略。在此基础上，提出了如下方法来调整MOF衍生物的电磁参数，以实现良好的电磁能量耗散：(1)改变金属和配体以调节前驱体的化学成分和形貌；(2)控制热解参数(包括温度、升温速度和气体气氛)以控制衍生物的结构和组分；(3)与增强相复合，包括碳纳米材料、金属或其他MOF。

关键词:

Invited Review

A literature review of MOF derivatives of electromagnetic wave absorbers mainly based on pyrolysis

+ Author Affiliations

1)
Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Nanjing Forestry University, Nanjing 210037, China
2)
College of Materials Science and Engineering, Nanjing Forestry University, Nanjing 210037, China
3)
Henan Science & Technology Exchange Center with Foreign Countries, Zhengzhou 450000, China
4)
College of Engineering, University of Georgia, Athens 30605, USA

*The authors contributed equally to this paper.

Corresponding authors:
Zhichao Lou E-mail: zc-lou2015@njfu.edu.cn

Yanjun Li E-mail: nfcm2018@163.com
Received: 25 July 2022; Revised: 23 October 2022; Accepted: 24 October 2022; Available online: 25 October 2022

Abstract

Abstract

Growing electromagnetic pollution has plagued researchers in the field of electromagnetic (EM) energy dissipation for many years; it is increasingly important to solve this problem efficiently. Metal–organic frameworks (MOFs), a shining star of functional materials, have attracted great attention for their advantages, which include highly tunable porosity, structure, and versatility. MOF-derived electromagnetic wave (EMW) absorbers, with advantages such as light weight, thin matching thickness, strong capacity, and wide effective bandwidth, are widely reported. However, current studies lack a systematic summary of the ternary synergistic effects of the precursor component–structure–EMW absorption behavior of MOF derivatives. Here we describe in detail the electromagnetic (EM) energy dissipation mechanism and strategy for preparing MOF-derived EMW absorbers. On the basis of this description, the following means are suggested for adjusting the EM parameters of MOF derivatives, achieving excellent EM energy dissipation: (1) changing the metal and ligands to regulate the chemical composition and morphology of the precursor, (2) controlling pyrolysis parameters (including temperature, heating rate, and gas atmosphere) to manipulate the structure and components of derivatives, and (3) compounding with enhancement phases, including carbon nanomaterials, metals, or other MOFs.
- metal organic framework;
- microstructure;
- magnetic–dielectric synergy;
- electromagnetic wave absorption

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