Bo Wang, Jiawei Li, Zhihui Xie, Gengjie Wang,  and Gang Yu, High corrosion and wear resistant electroless Ni–P gradient coatings on aviation aluminum alloy parts, Int. J. Miner. Metall. Mater., 31(2024), No. 1, pp. 155-164. https://doi.org/10.1007/s12613-023-2689-3
Cite this article as:
Bo Wang, Jiawei Li, Zhihui Xie, Gengjie Wang,  and Gang Yu, High corrosion and wear resistant electroless Ni–P gradient coatings on aviation aluminum alloy parts, Int. J. Miner. Metall. Mater., 31(2024), No. 1, pp. 155-164. https://doi.org/10.1007/s12613-023-2689-3
Research Article

High corrosion and wear resistant electroless Ni–P gradient coatings on aviation aluminum alloy parts

+ Author Affiliations
  • Corresponding authors:

    Zhihui Xie    E-mail: zhxie@cwnu.edu.cn

    Gang Yu    E-mail: yuganghnu@163.com

  • Received: 1 February 2023Revised: 25 April 2023Accepted: 5 June 2023Available online: 6 June 2023
  • A Ni–P alloy gradient coating consisting of multiple electroless Ni–P layers with various phosphorus contents was prepared on the aviation aluminum alloy. Several characterization and electrochemical techniques were used to characterize the different Ni–P coatings’ morphologies, phase structures, elemental compositions, and corrosion protection. The gradient coating showed good adhesion and high corrosion and wear resistance, enabling the application of aluminum alloy in harsh environments. The results showed that the double zinc immersion was vital in obtaining excellent adhesion (81.2 N). The optimal coating was not peeled and shredded even after bending tests with angles higher than 90° and was not corroded visually after 500 h of neutral salt spray test at 35°C. The high corrosion resistance was attributed to the misaligning of these micro defects in the three different nickel alloy layers and the amorphous structure of the high P content in the outer layer. These findings guide the exploration of functional gradient coatings that meet the high application requirement of aluminum alloy parts in complicated and harsh aviation environments.
  • loading
  • [1]
    S. Basak, P. Biswas, S. Patra, H. Roy, and M.K. Mondal, Effect of TiB2 and Al3Ti on the microstructure, mechanical properties and fracture behaviour of near eutectic Al–12.6Si alloy, Int. J. Miner. Metall. Mater., 28(2021), No. 7, p. 1174. doi: 10.1007/s12613-020-2070-8
    [2]
    Y. Jafari-Tarzanagh, D. Seifzadeh, A. Khodayari, and R. Samadianfard, Active corrosion protection of AA2024 aluminum alloy by sol–gel coating containing inhibitor-loaded mesoporous SBA-15, Prog. Org. Coat., 173(2022), art. No. 107166. doi: 10.1016/j.porgcoat.2022.107166
    [3]
    Y.J. Tarzanagh, D. Seifzadeh, Z. Rajabalizadeh, A. Habibi-Yangjeh, A. Khodayari, and S. Sohrabnezhad, Sol–gel/MOF nanocomposite for effective protection of 2024 aluminum alloy against corrosion, Surf. Coat. Technol., 380(2019), art. No. 125038. doi: 10.1016/j.surfcoat.2019.125038
    [4]
    S. Yadav, S.P. Tewari, J.K. Singh, and S.C. Ram, Effects of mechanical vibration on the physical, metallurgical and mechanical properties of cast A308 (LM21) aluminum alloy, Int. J. Miner. Metall. Mater., 29(2022), No. 6, p. 1206. doi: 10.1007/s12613-020-2209-7
    [5]
    Z. Shao, L. Cui, L.J. Yang, et al., Microstructure and mechanical properties of friction pull plug welding for 2219-T87 aluminum alloy with tungsten inert gas weld, Int. J. Miner. Metall. Mater., 29(2022), No. 6, p. 1216. doi: 10.1007/s12613-020-2222-x
    [6]
    C. Duraipandi, A. Khan M, J.J.T. Winowlin, N.M. Ghazaly, and P.M. Mashinini, Solid particle erosion studies of thermally deposited alumina–titania coatings on an aluminum alloy, Int. J. Miner. Metall. Mater., 28(2021), No. 7, p. 1186. doi: 10.1007/s12613-020-2099-8
    [7]
    H. Ebrahimzadeh, H. Farhangi, S.A.A.A. Mousavi, and A. Ghahramani, Microstructural analyses of aluminum–magnesium–silicon alloys welded by pulsed Nd:YAG laser welding, Int. J. Miner. Metall. Mater., 27(2020), No. 5, p. 660. doi: 10.1007/s12613-020-2027-y
    [8]
    A.G.G. Gutiérrez, M.A. Pech-Canul, and P.J. Sebastian, Zincating effect on corrosion resistance of electroless Ni–P coating on aluminum alloy 6061, Fuel Cells, 17(2017), No. 6, p. 770. doi: 10.1002/fuce.201600212
    [9]
    S. Nezamdoust and D. Seifzadeh, rGO@APTES/hybrid sol–gel nanocomposite for corrosion protection of 2024 aluminum alloy, Prog. Org. Coat., 109(2017), p. 97. doi: 10.1016/j.porgcoat.2017.04.022
    [10]
    I. Fatima, O. Fayyaz, M.M. Yusuf, A. Al Ashraf, and R.A. Shakoor, Enhanced electrochemical and mechanical performance of BN reinforced Ni–P based nanocomposite coatings, Diam. Relat. Mater., 130(2022), art. No. 109454. doi: 10.1016/j.diamond.2022.109454
    [11]
    M.H. Sliem, O. Fayyaz, R.A. Shakoor, et al., The influence of different preparation methods on the erosion behavior of NiP–ZrO2 nanocomposite coating, Tribol. Int., 178(2023), art. No. 108014. doi: 10.1016/j.triboint.2022.108014
    [12]
    C.O. Osifuye, A.P.I. Popoola, C.A. Loto, and D.T. Oloruntoba, Effect of bath parameters on electroless Ni–P and Zn–P deposition on 1045 steel substrate, Int. J. Electrochem. Sci., 9(2014), No. 11, p. 6074. doi: 10.1016/S1452-3981(23)10871-6
    [13]
    Z.H. Xie, D. Li, Z. Skeete, A. Sharma, and C.J. Zhong, Nanocontainer-enhanced self-healing for corrosion-resistant Ni coating on Mg alloy, ACS Appl. Mater. Interfaces, 9(2017), No. 41, p. 36247. doi: 10.1021/acsami.7b12036
    [14]
    Y.Q. Li, Y.J. Ouyang, R. Fang, et al., A nickel-underlayer/LDH-midlayer/siloxane-toplayer composite coating for inhibiting galvanic corrosion between Ni layer and Mg alloy, Chem. Eng. J., 430(2022), art. No. 132776. doi: 10.1016/j.cej.2021.132776
    [15]
    Z.W. Song, Z.H. Xie, L.F. Ding, Y.J. Zhang, and X.Y. Hu, Preparation of corrosion-resistant MgAl-LDH/Ni composite coating on Mg alloy AZ31B, Colloids Surf. A, 632(2022), art. No. 127699. doi: 10.1016/j.colsurfa.2021.127699
    [16]
    M. Kocabaş, C. Örnek, M. Curioni, and N. Cansever, Nickel fluoride as a surface activation agent for electroless nickel coating of anodized AA1050 aluminum alloy, Surf. Coat. Technol., 364(2019), p. 231. doi: 10.1016/j.surfcoat.2019.03.003
    [17]
    F. Delaunois, J.P. Petitjean, P. Lienard, and M. Jacob-Duliere, Autocatalytic electroless nickel–boron plating on light alloys, Surf. Coat. Technol., 124(2000), No. 2-3, p. 201. doi: 10.1016/S0257-8972(99)00621-0
    [18]
    X.C. Wei, J.B. Wang, X.M. Zhang, and X.G. Wang, Study on the development of pretreatment processes of electroless nickel plating on Al alloy surface, Mater. Sci. Forum, 809-810(2014), p. 412. doi: 10.4028/www.scientific.net/MSF.809-810.412
    [19]
    S. Wernick, R. Pinner, and P.G. Sheasby, The Surface Treatment and Finishing of Aluminum and Its Alloys, 6th ed., ASM International Materials Park, OH, 2001.
    [20]
    C.H. Zhang, X.M. Huang, N. Sheng, and L.L. Gao, A zinc dipping technique for Mg–16Li–5Al–0.5RE alloy at room temperature, Mater. Corros., 64(2013), No. 6, p. 509. doi: 10.1002/maco.201206535
    [21]
    I.S. Othman, M.J. Starink, and S.C. Wang, Impact of single and double zincating treatment on adhesion of electrodeposited nickel coating on aluminium alloy 7075, J. Adv. Manuf. Technol., 12(2018), p. 179.
    [22]
    D.D.N. Singh and R. Ghosh, Electroless nickel–phosphorus coatings to protect steel reinforcement bars from chloride induced corrosion, Surf. Coat. Technol., 201(2006), No. 1-2, p. 90. doi: 10.1016/j.surfcoat.2005.10.045
    [23]
    J.D. Lin and C.T. Chou, The influence of phosphorus content on the microstructure and specific capacitance of etched electroless Ni–P coatings, Surf. Coat. Technol., 368(2019), p. 126. doi: 10.1016/j.surfcoat.2019.04.009
    [24]
    Y.F. Li, K. Zhang, M.M. Zhang, T.T. Wu, P. Cao, and W. Gao, Preparation of electroless Ni–P alloy coating with medium temperature and low phosphorus content, Int. J. Mod. Phys. B, 34(2020), art. No. 2040044. doi: 10.1142/S0217979220400445
    [25]
    E. Georgiza, J. Novakovic, and P. Vassiliou, Characterization and corrosion resistance of duplex electroless Ni–P composite coatings on magnesium alloy, Surf. Coat. Technol., 232(2013), p. 432. doi: 10.1016/j.surfcoat.2013.05.047
    [26]
    A. Hadipour, M. Rahsepar, and H. Hayatdavoudi, Fabrication and characterisation of functionally graded Ni–P coatings with improved wear and corrosion resistance, Surf. Eng., 35(2019), No. 10, p. 883. doi: 10.1080/02670844.2018.1539295
    [27]
    F.L. Zheng, H.S. Chen, Y.Q. Zhang, W.X. Wang, and H.H. Nie, Microstructure evolution and corrosion resistance of AZ31 magnesium alloy tube by stagger spinning, Int. J. Miner. Metall. Mater., 29(2022), No. 7, p. 1361. doi: 10.1007/s12613-021-2396-x
    [28]
    L.D. Ma, G. Lü, and X.L. Shen, An investigation of chemically deposited Ni–P alloys by EXAFS and XRD, Chin. J. Chem., 8(1990), No. 3, p. 239. doi: 10.1002/cjoc.19900080308
    [29]
    M. Rahsepar, F. Mohebbi, and H. Hayatdavoudi, Synthesis and characterization of inhibitor-loaded silica nanospheres for active corrosion protection of carbon steel substrate, J. Alloys Compd., 709(2017), p. 519. doi: 10.1016/j.jallcom.2017.03.104
    [30]
    H. Hayatdavoudi and M. Rahsepar, A mechanistic study of the enhanced cathodic protection performance of graphene-reinforced zinc rich nanocomposite coating for corrosion protection of carbon steel substrate, J. Alloys Compd., 727(2017), p. 1148. doi: 10.1016/j.jallcom.2017.08.250
    [31]
    H. Hayatdavoudi and M. Rahsepar, Smart inhibition action of layered double hydroxide nanocontainers in zinc-rich epoxy coating for active corrosion protection of carbon steel substrate, J. Alloys Compd., 711(2017), p. 560. doi: 10.1016/j.jallcom.2017.04.044
    [32]
    H. Luo, M. Leitch, Y. Behnamian, Y.S. Ma, H.B. Zeng, and J.L. Luo, Development of electroless Ni–P/nano-WC composite coatings and investigation on its properties, Surf. Coat. Technol., 277(2015), p. 99. doi: 10.1016/j.surfcoat.2015.07.011
    [33]
    E.M. Fayyad, A.M. Abdullah, M.K. Hassan, A.M. Mohamed, G. Jarjoura, and Z. Farhat, Recent advances in electroless-plated Ni–P and its composites for erosion and corrosion applications: A review, Emergent Mater., 1(2018), No. 1, p. 3.
    [34]
    U. Ma and D.T. Gawne, Wear of electroless nickel–phosphorus coatings, Trans. IMF, 63(1985), No. 1, p. 64. doi: 10.1080/00202967.1985.11870709
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索

    Figures(11)  / Tables(3)

    Share Article

    Article Metrics

    Article Views(478) PDF Downloads(39) Cited by()
    Proportional views

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return