Abstract:
Metal-halide perovskites have been successfully utilized in high-sensitivity direct X-ray detection, and the further integration of perovskites with pixel chips is crucial for X-ray imaging. In this study, an ingenious interface-bonding strategy is applied to integrate a polycrystalline CsPbBr
3 wafer with a thin-film transistor (TFT) array. A polyimide-CsPbBr
3 composite binder with satisfactory mechanical adhesion and optoelectronic properties is synthesized and used to integrate a freestanding CsPbBr
3 wafer with a TFT array. Under low-temperature annealing, interface reconstruction occurs with the
in-situ formation of a homogeneous bridging structure between the CsPbBr
3 wafer and TFT array, achieving a multichannel X-ray imaging detector. The X-ray detector exhibits a high sensitivity of 4310 µC·Gy
−1·cm
−2 and low detection limit of 442 nGy·s
−1. The resulting imaging panel with pixels offers a satisfactory spatial resolution (2.2 LP·mm
−1) X-ray imaging.