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Invited Review

Research progress of electrochemical impedance technique applied in the high-capacity lithium-ion battery

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  • Received: 23 July 2020Revised: 28 October 2020Accepted: 2 November 2020Available online: 4 November 2020
  • The world’s energy system is changing dramatically. The Li ion battery, as a powerful and highly effective energy storage technique, is critical to the new-energy revolution for their continuous expanding application in the electric vehicles and the electric grids. Over the whole lifetime of the batteries, it is essential to monitor their state of health. It is not only for the mileage prediction, safety management in the running electric vehicle, but also for an “end-of-life” evaluation to repurpose the power batteries. Electrochemical impedance spectroscopy (EIS) has been widely used to quickly and non-destructively diagnose the health state of batteries. In this review, we have outlined the working principles of several electrochemical impedance techniques, and further evaluated its application prospects to achieve the goal of non-destructive testing of battery health. We believe that EIS can scientifically and reasonably perform real-time monitoring and evaluation of electric vehicle power batteries in the future, and mentions the important role of vehicle safety and battery gradient utilization.
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Research progress of electrochemical impedance technique applied in the high-capacity lithium-ion battery

  • Corresponding author:

    Xin-dong Wang    E-mail: echem@ustb.edu.cn

  • 1. Department of Physical Chemistry, School of Metallurgical and Ecological Engineering, University of Science and Technology Beijing, Beijing 100083, China
  • 2. China Electric Power Research Institute, Beijing 100192, China
  • 3. Electric Power Research Institute, State Grid Shanghai Municipal Electric Power Company, Shanghai 200437, China

Abstract: The world’s energy system is changing dramatically. The Li ion battery, as a powerful and highly effective energy storage technique, is critical to the new-energy revolution for their continuous expanding application in the electric vehicles and the electric grids. Over the whole lifetime of the batteries, it is essential to monitor their state of health. It is not only for the mileage prediction, safety management in the running electric vehicle, but also for an “end-of-life” evaluation to repurpose the power batteries. Electrochemical impedance spectroscopy (EIS) has been widely used to quickly and non-destructively diagnose the health state of batteries. In this review, we have outlined the working principles of several electrochemical impedance techniques, and further evaluated its application prospects to achieve the goal of non-destructive testing of battery health. We believe that EIS can scientifically and reasonably perform real-time monitoring and evaluation of electric vehicle power batteries in the future, and mentions the important role of vehicle safety and battery gradient utilization.

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